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Molecular beam epitaxy

<Abstract>

Molecular beam epitaxy (MBE) is a process for growing thin, epitaxial films of a wide variety of

materials,ranging from oxides to semiconductors to metals. It was first applied to the growth

of compound semiconductors.That is still the most common usage, in large part because of

the high technological value of such materials to theelectronics industry. In this process

beams of atoms or molecules in an ultra-high vacuum environment are incidentupon a heated

crystal that has previously been processed to produce a nearly atomically clean surface.

The arriving constituent atoms form a crystalline layer in registry with the substrate, i.e., an

epitaxial film. These films areremarkable because the composition can be rapidly changed,

producing crystalline interfaces that are almost atomically abrupt. Thus, it has been possible

to produce a large range of unique structures, including quantum well devices,superlattices,

lasers, etc., all of which benefit from the precise control of composition during growth.

Because of the cleanliness of the growth environment and because of the precise control

over composition, MBE structures closely approximate the idealized models used in solid

state theory.

This discussion is intended as an introduction to the concept and the experimental procedures

used in MBE growth. The refinement of experimental procedures has been the key to the

successful fabrication of electronically significant devices, which in turn has generated the

widespread interest in the MBE as a research tool. MBE experiments have provided a wealth

of new information bearing on the general mechanisms involved in epitaxial growth, since

many of the phenomena initially observed during MBE have since been repeated using other

crystal growth processes. We also summarize the general types of layered structures that have

contributed to the rapid expansion of interest in MBE and its various offshoots. Finally we

consider some of the problems that remain in the growth of heteroepitaxial structures, specifically,

the problem of mismatch in lattice constant between layers and between layer and substrate.

The discussion is phenomenological, not theoretical; MBE has been primarily an experimental approach based on simple concepts.

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