Strengthening and toughening mechanisms in graphene-Al nanolaminated composite micro-pillars
<Abstract>
Uniaxial compression tests were carried out on micro-pillars fabricated from
nanolaminated graphene (reduced graphene oxide, RGO)-Al composites of
different RGO concentrations and laminate orientations (the angle between
laminate planes and the pillar axis). It was found that the strengthening capability
of RGO can be enhanced by either orienting the RGO layers parallel with the
loading direction or raising the RGO concentration. The stress–strain response
of the micro-pillars was populated with discrete bursts, and the stress increments
of the bursts scaled with the RGO concentration, regardless of the laminate
orientation relative to the loading direction. These observations were interpreted
by the variation in the load-bearing capacity of RGO in different laminate
orientations, the dislocation annihilation at the RGO/Al interface, and a crack
deflection mechanism provided by the robust RGO/Al interface that toughened
the composites. This work underscores the importance of structural design and
control in the stiffening, strengthening, and toughening of metal matrix composites,
and the methodology developed may be applied to other composites with
microstructural heterogeneity to probe their specific mechanical behaviors
and structure-property correlations.